Abstract:5 . -The title compound is synthesized from the elements by a self-flux route (700°C, 10 h) and by solid state reaction (500°C, 10 d). The samples are characterized by single crystal XRD, magnetic measurements, and electronic band structure calculations employing FPLO, LMTO, and extended Hueckel tight-binding methods. The compound crystallizes in the tetragonal space group P4/mbm with Z = 2. The structure exhibits a three-dimensional Ga network made up of two crystallographically different types of Ga atoms. M… Show more
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