Abstract.We give the definitions of exact and approximate controllability for linear and nonlinear Schrödinger equations, review fundamental criteria for controllability and revisit a classical "No-go" result for evolution equations due to Ball, Marsden and Slemrod. In Section 2 we prove corresponding results on non-controllability for the linear Schrödinger equation and distributed additive control, and we show that the Hartree equation of quantum chemistry with bilinear control (E(t) · x)u is not controllable in finite or infinite time. Finally, in Section 3, we give criteria for additive controllability of linear Schrödinger equations, and we give a distributed additive controllability result for the nonlinear Schrödinger equation if the data are small.Mathematics Subject Classification. 35Q40, 35Q55, 81Q99, 93B05.