2024
DOI: 10.1021/acs.inorgchem.4c02337
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Conversion of Carbon Dioxide into a Series of CBxOy Compounds Mediated by LaB3,4O2 Anions: Synergy of the Electron Transfer and Lewis Pair Mechanisms to Construct B–C Bonds

Feng-Xiang Zhang,
Ming Wang,
Jia-Bi Ma

Abstract: Converting CO 2 into value-added products containing B−C bonds is a great challenge, especially for multiple B−C bonds, which are versatile building blocks for organoborane chemistry. In the condensed phase, the B−C bond is typically formed through transition metal-catalyzed direct borylation of hydrocarbons via C−H bond activation or transition metal-catalyzed insertion of carbenes into B−H bonds. However, excessive amounts of powerful boryl reagents are required, and products containing B−C bonds are complex… Show more

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