Dynamic Coordination Engineering of Z‐Scheme (FFV)2PdCl2/C3N4 Heterojunction for Superior Photocatalytic Hydrogen Evolution
Jiapeng Xu,
Dong Liu,
Xinming Li
et al.
Abstract:Realizing highly efficient photocatalytic hydrogen evolution reaction (HER) is a key challenge. Herein, a (FFV)2PdCl2 complex is developed with dynamic coordination engineering between the PdII site and Fluoflavin (FFV) ligands, and couple it with graphite carbon nitride (g‐C3N4) ultrathin nanosheets to construct a novel Z‐scheme heterojunction ((FFV)2PdCl2/C3N4). The resultant heterojunction delivers a HER activity of 648 µmol h−1 under visible light (λ ≥ 400 nm) illumination and an apparent quantum yield up… Show more
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