Electrochemical urea synthesis

Kohlhaas, Yannik; Tschauder, Yannick S.; Plischka, Wenzel; Simon, Ulrich; Eichel, Rüdiger-A.; Wessling, Matthias; Keller, Robert

doi:10.1016/j.joule.2024.04.004

Joule

2024

DOI: 10.1016/j.joule.2024.04.004

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Electrochemical urea synthesis

Yannik Kohlhaas,

Yannick S. Tschauder,

Wenzel Plischka

et al.

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2024

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Cited by 4 publications

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Heterogeneous electrocatalytic synthesis of nitrogenous organic compounds using inorganic nitrogen sources

Wang,

Li,

Besenbacher

et al. 2024

Nano Materials Science

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Heterogeneous electrocatalytic synthesis of nitrogenous organic compounds using inorganic nitrogen sources

Wang,

Li,

Besenbacher

et al. 2024

Nano Materials Science

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Enhanced Electrocatalytic Urea Synthesis over Iron-Doped InOOH Nanosheets under Ambient Conditions

Cai,

Wang,

Meng

et al. 2024

Inorg. Chem.

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Ambient urea synthesis via C−N coupling from CO 2 and nitrate reduction offers an attractive alternative to the Bosch-Meiser route, but it is hindered by the lack of efficient catalysts. Herein, we report that Fe-doped InOOH nanosheets effectively catalyze the coreduction of CO 2 and nitrate, giving a high Faradaic Efficiency of 26.9%, a yield rate of 980.6 μg h −1 mg cat.−1 , and a good durability. Theoretical calculations further elucidate that iron dopants can tailor the reactivity of the In site, facilitating the hydrogenation of the key *CO 2 NH 2 intermediate and suppressing the hydrogen production with a higher energy barrier.

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Efficient electrocoupling of CO₂ and N₂ to urea by a gas-penetrable Bi nanosheet-wrapped Cu hollow fiber

Wang,

Wang

et al. 2024

Chem. Commun.

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Electrochemical urea synthesis

Cited by 4 publications

References 101 publications

Heterogeneous electrocatalytic synthesis of nitrogenous organic compounds using inorganic nitrogen sources

Heterogeneous electrocatalytic synthesis of nitrogenous organic compounds using inorganic nitrogen sources

Enhanced Electrocatalytic Urea Synthesis over Iron-Doped InOOH Nanosheets under Ambient Conditions

Efficient electrocoupling of CO₂ and N₂ to urea by a gas-penetrable Bi nanosheet-wrapped Cu hollow fiber

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Electrochemical urea synthesis

Cited by 4 publications

References 101 publications

Heterogeneous electrocatalytic synthesis of nitrogenous organic compounds using inorganic nitrogen sources

Heterogeneous electrocatalytic synthesis of nitrogenous organic compounds using inorganic nitrogen sources

Enhanced Electrocatalytic Urea Synthesis over Iron-Doped InOOH Nanosheets under Ambient Conditions

Efficient electrocoupling of CO2 and N2 to urea by a gas-penetrable Bi nanosheet-wrapped Cu hollow fiber

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Product

Resources

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Efficient electrocoupling of CO₂ and N₂ to urea by a gas-penetrable Bi nanosheet-wrapped Cu hollow fiber