2022
DOI: 10.26434/chemrxiv-2022-g9bvt
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Elucidating the Impact of Structural Parameters on the Glass Transition Temperatures of Bottlebrush Polymers

Abstract: The glass transition of branched polymers is determined by multiple structural parameters that dictate their inter- and intramolecular interactions, and ultimately, their molecular packing in the amorphous phase. Here we examined the impact of side chain length, backbone length, molecular weight composition, and topology on the glass transition behavior of bottlebrush polymers. Through examining precision bottlebrush polymer libraries (PBP, ĐSC = 1.0), we find the infinite molecular weight Tg is reached at a s… Show more

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