2024
DOI: 10.1002/aenm.202402091
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Enhanced Interfacial Conduction in Low‐Cost NaAlCl4 Composite Solid Electrolyte for Solid‐State Sodium Batteries

Erick Ruoff,
Steven Kmiec,
Arumugam Manthiram

Abstract: All‐solid‐state sodium batteries offer the advantage of both sustainability and safety. Solid‐state electrolytes play a key role, and an oxygen‐incorporated NaAlCl4 composite electrolyte is presented with a high ambient‐temperature ionic conductivity of > 0.1 mS cm−1. The electrolyte synthesized with a mechanochemical reaction consists of in situ‐formed Al2O3 nanoparticles that provide enhanced conduction through an oxychloride phase at the interface. Magic angle spinning nuclear magnetic resonance spectros… Show more

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