Enhanced lubrication and photothermal conversion <i>via</i> dynamically reversible supramolecular oil gels filled with MXene@<i>m</i>GLM composites

Cui, Yuhong; Wang, Tiantian; Jin, Guangkai; Wang, Shiyuan; Liu, Shujuan; Ye, Qian; Zhou, Feng; Liu, Weimin

doi:10.1039/d4ta03064h

J. Mater. Chem. A

2024

DOI: 10.1039/d4ta03064h

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Enhanced lubrication and photothermal conversion via dynamically reversible supramolecular oil gels filled with MXene@mGLM composites

Yuhong Cui,

Tiantian Wang,

Guangkai Jin

et al.

Abstract: Herein, we have successfully fabricated supramolecular oil gels using a combination of MXene@mGLM composites and gelator 12-hydroxystearic acid (12-HSA) in base oil polyalphaolefin (PAO) through non-covalent bonding interactions. Initially, the...

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Schottky Interface Engineering in Ti₃C₂T_x/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers

Cui,

Ru,

Zhang

et al. 2024

Adv Funct Materials

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With the rapid advancement of wearable electronics, soft robotics, and camouflage technologies, there is an urgent demand for flexible, multifunctional electromagnetic wave absorbing materials. Traditional absorbers, including metal‐ and carbon‐based materials, often lack the flexibility required for such applications. In this work, a novel strategy is proposed for developing a flexible absorber by combining a conductive filler with a Schottky heterogeneous interface and a polymer network framework. Ti3C2Tx MXene is modified with ZnS via a low‐temperature hydrothermal method, forming a Ti3C2Tx/ZnS composite. This composite is subsequently embedded in a copolymer matrix of polyvinyl alcohol (PVA) and acrylamide (AAm), dispersed in a binary water‐glycerol solution. The Schottky interface between Ti3C2Tx and ZnS enhances electron transfer at the heterophase boundary, significantly improving interface polarisation. Simultaneously, interactions between water and glycerol restrict the rotation of polar molecules under external electromagnetic fields, optimising polarisation loss within the gel. Experimental results demonstrate that the Ti3C2Tx/ZnS gel achieves a minimum reflection loss (RLmin) of −43.76 dB at 8.79 GHz, with an effective absorption bandwidth (EAB) covering the entire X‐band. Additionally, the gel exhibit exceptional stretchability, frost resistance, shape adaptability, and photothermal conversion properties.

show abstract

Schottky Interface Engineering in Ti₃C₂T_x/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers

Cui,

Ru,

Zhang

et al. 2024

Adv Funct Materials

View full text Add to dashboard Cite

show abstract

Fabrication of ionic liquid-functionalized carbon dots as lubricant additive for friction and wear reduction

Xue,

Zhang,

Wang

et al. 2025

Tribology International

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Fabrication of functional N, S co-doped MXene for enhance tribological performance

Cui,

Chen,

Wang

et al. 2025

Tribology International

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Enhanced lubrication and photothermal conversion via dynamically reversible supramolecular oil gels filled with MXene@mGLM composites

Abstract: Herein, we have successfully fabricated supramolecular oil gels using a combination of MXene@mGLM composites and gelator 12-hydroxystearic acid (12-HSA) in base oil polyalphaolefin (PAO) through non-covalent bonding interactions. Initially, the...

Cited by 5 publications

References 48 publications

Schottky Interface Engineering in Ti₃C₂T_x/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers

Schottky Interface Engineering in Ti₃C₂T_x/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers

Fabrication of ionic liquid-functionalized carbon dots as lubricant additive for friction and wear reduction

Fabrication of functional N, S co-doped MXene for enhance tribological performance

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Product

Resources

About

Enhanced lubrication and photothermal conversion via dynamically reversible supramolecular oil gels filled with MXene@mGLM composites

Abstract: Herein, we have successfully fabricated supramolecular oil gels using a combination of MXene@mGLM composites and gelator 12-hydroxystearic acid (12-HSA) in base oil polyalphaolefin (PAO) through non-covalent bonding interactions. Initially, the...

Cited by 5 publications

References 48 publications

Schottky Interface Engineering in Ti3C2Tx/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers

Schottky Interface Engineering in Ti3C2Tx/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers

Fabrication of ionic liquid-functionalized carbon dots as lubricant additive for friction and wear reduction

Fabrication of functional N, S co-doped MXene for enhance tribological performance

Contact Info

Product

Resources

About

Schottky Interface Engineering in Ti₃C₂T_x/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers

Schottky Interface Engineering in Ti₃C₂T_x/ZnS Organic Hydrogels for High‐Performance Multifunctional Flexible Absorbers