Enhancing perovskite solar cell performance through PbI<sub>2</sub><i>in situ</i> passivation using a one-step process: experimental insights and simulations

Rabhi, Selma; Sekar, Karthick; Kalna, Karol; Hidouri, Tarak; Samajdar, Dip Prakash; Ravidas, Babban Kumar; Bencherif, Hichem; Fornari, Roberto; Albaidani, Kouloud; Hossain, M. Khalid

doi:10.1039/d4ra06193d

RSC Adv.

2024

DOI: 10.1039/d4ra06193d

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Enhancing perovskite solar cell performance through PbI₂in situ passivation using a one-step process: experimental insights and simulations

Selma Rabhi,

Karthick Sekar,

Karol Kalna

et al.

Abstract: The new architecture of MAPbI3-based solar cells with photovoltaic parameters. The inset shows a new schematic design of the n-i-p structure for the PSC used in SCAPS simulation: AZO/SnO2/MAPbI3 with excess PbI2/spiro-OMeTAD/IZO.

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Role of Ag Nanowires: MXenes in Optimizing Flexible, Semitransparent Bifacial Inverted Perovskite Solar Cells for Building‐Integrated Photovoltaics: A SCAPS‐1D Modeling Approach

Alathlawi,

Rabhi,

Hidouri

et al. 2024

Advcd Theory and Sims

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Semi‐transparent perovskite solar cells (ST‐PSCs) offer a promising pathway for use in building integrated photovoltaic (BIPV) systems instead of conventional panels’ roofs. Furthermore, their potential for bifacial operation, allowing light absorption from both sides, creates new opportunities for their integration as solar cells windows, and greatly improves energy harvesting capacities. This combination of bifaciality and flexibility enhances their efficiency and adaptability, making them well‐suited for integration into various architectural elements. Herein, in this study, the performance of 40 different configurations of bifacial flexible semi‐transparent inverted perovskite solar cells (BF‐STIPSCs) is explored. Using SCAPS‐1D (version 3.3.11), a 3D‐perovskite (PVK) absorber layer is modeled and combined with polymer‐based electron transport layers (ETLs) such as C60 and BCP, along with innovative hole transport layers (HTLs) including D‐PBTTT‐14, Me‐4PACz, NiOx, PANI, Poly‐TPD, PATAA, SrCuO2, V2O5. Various transparent conductive oxides (TCOs) including IWO, ITO, and FTO, and flexible substrates such as silver nanowires (AgNWs) with two‐dimensional transition carbide (MXene: T2CF2) are also examined for their effects on the cells' bifaciality, transparency, and stability. Among the configurations, PET/Ag NWs:MXenes /SrCuO2/(FAPbI3)0.95(MAPbBr3)0.05/C60/BCP/FTO is identified as a high‐performance structure, achieving a power conversion efficiency (PCE) of ≈26%, along with enhanced resilience to temperature variations. These results hold great promise for the integration of perovskite‐based semitransparent bifacial flexible solar cells into real‐world applications.

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Role of Ag Nanowires: MXenes in Optimizing Flexible, Semitransparent Bifacial Inverted Perovskite Solar Cells for Building‐Integrated Photovoltaics: A SCAPS‐1D Modeling Approach

Alathlawi,

Rabhi,

Hidouri

et al. 2024

Advcd Theory and Sims

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Enhancing perovskite solar cell performance through PbI₂in situ passivation using a one-step process: experimental insights and simulations

Abstract: The new architecture of MAPbI3-based solar cells with photovoltaic parameters. The inset shows a new schematic design of the n-i-p structure for the PSC used in SCAPS simulation: AZO/SnO2/MAPbI3 with excess PbI2/spiro-OMeTAD/IZO.

Cited by 1 publication

References 81 publications

Role of Ag Nanowires: MXenes in Optimizing Flexible, Semitransparent Bifacial Inverted Perovskite Solar Cells for Building‐Integrated Photovoltaics: A SCAPS‐1D Modeling Approach

Role of Ag Nanowires: MXenes in Optimizing Flexible, Semitransparent Bifacial Inverted Perovskite Solar Cells for Building‐Integrated Photovoltaics: A SCAPS‐1D Modeling Approach

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Enhancing perovskite solar cell performance through PbI2in situ passivation using a one-step process: experimental insights and simulations

Abstract: The new architecture of MAPbI3-based solar cells with photovoltaic parameters. The inset shows a new schematic design of the n-i-p structure for the PSC used in SCAPS simulation: AZO/SnO2/MAPbI3 with excess PbI2/spiro-OMeTAD/IZO.

Cited by 1 publication

References 81 publications

Role of Ag Nanowires: MXenes in Optimizing Flexible, Semitransparent Bifacial Inverted Perovskite Solar Cells for Building‐Integrated Photovoltaics: A SCAPS‐1D Modeling Approach

Role of Ag Nanowires: MXenes in Optimizing Flexible, Semitransparent Bifacial Inverted Perovskite Solar Cells for Building‐Integrated Photovoltaics: A SCAPS‐1D Modeling Approach

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Enhancing perovskite solar cell performance through PbI₂in situ passivation using a one-step process: experimental insights and simulations