Catal. Sci. Technol.
 2023
DOI: 10.1039/d3cy00392b
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Entropic influence on the generation of Fe(iv)O species at mononuclear Fe(ii) sites in metal–organic frameworks

Fernan Saiz,
Leonardo Bernasconi

Abstract: We study the oxidation of mononuclear Fe(II) centers in the metal-organic framework MOF-74 in the presence of nitric oxide (NO), nitrogen dioxide (NO$_2$), nitrous oxide (N$_2$O), dinitrous dioxide (N$_2$O$_2$), oxygen...

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