Experimental study on the scale-up of a multi-ring inclined nozzle spout-fluid bed by electrical capacitance tomography

Abstract

Scale-up studies of fluidized beds are important for numerous fields. Fluidization in a multi-ring inclined nozzle spout-fluid bed (MRIN spout-fluid bed) is one of the most critical factors that affect the coating efficiency and uniformity of tri-structural isotropic (TRISO) nuclear particles in the fluidized bed chemical vapor deposition (FB-CVD) process. In this work, the flow pattern similarity principle was proposed to scale up a specially designed spout-fluid bed, which was aimed at maintaining the gas-solid contact efficiency, and was validated by electrical capacitance tomography (ECT) measurements. First, the traditional ECT method was developed for the specially designed MRIN spout-fluid bed according to the filling method. Then, the reconstruction algorithms were updated using the alternating direction multiplier method (ADMM) by introducing optimization constraints. The fluidization laws were investigated for different superficial gas velocities and distributor structures. We found that the gas distributor structure affected the merge point of the jets, which played an essential role in fluidization pattern changes. The statistically-based coefficient of variation (Cv) was proposed to distinguish the different flow patterns. Multi-ring spouting was then selected as a typical flow pattern for good fluidization and mixing, where the Cv ranged from 0.25 to 0.65. Then, the optimal design principles for the enlarged spout-fluid bed gas distributor were obtained. We determined that a smaller nozzle diameter (0.71d 0), larger nozzle spacing (1.12x 0), and slightly inclined angle (1.50θ 0) could improve fluidization, and that nozzle spacing was the most important factor. This study may be beneficial for the industrial design of the FB-CVD process and for the fabrication of high-density nuclear fuel particles. Additionally, it could be presented to a more general audience for scaling-up fluidized beds with a complex distributor, which would be beneficial for the fluidization research community.