2003
DOI: 10.1063/1.1574843
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External magnetic field effect on third-harmonic generation in Bi, Al-doped yttrium iron garnet

Abstract: The magnetic field effect on the third-harmonic generation (THG) in a Y1.5Bi1.5Fe3.8Al1.2O12 magnetic film was investigated. Applying a longitudinal external magnetic field rotated the polarization plane of the TH wave. The TH rotation angle was 4.1° at 2.67 eV (incoming wave: 0.89 eV) in a magnetic field of 1.0 kOe. Based on the symmetry analysis, the TH rotation was understood by an apparition of a magnetic term of χyxxx(3)(M) in a third-order nonlinear optical susceptibility.

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Cited by 9 publications
(6 citation statements)
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“…High surface and interface sensitivity along with large values of nonlinear magnetization-induced effects in SHG resulted in a fast development of this field of research during the last decade, when the advantages of the magnetization-sensitive SHG were demonstrated for clean surfaces and interfaces [3,4]. At the same time, higher-order (cubic) nonlinear magneto-optical effects were observed only recently [5] and the possibilities of this magnetization-sensitive probe for the diagnostics of magnetic structures are not clear till now.…”
Section: Introductionmentioning
confidence: 97%
“…High surface and interface sensitivity along with large values of nonlinear magnetization-induced effects in SHG resulted in a fast development of this field of research during the last decade, when the advantages of the magnetization-sensitive SHG were demonstrated for clean surfaces and interfaces [3,4]. At the same time, higher-order (cubic) nonlinear magneto-optical effects were observed only recently [5] and the possibilities of this magnetization-sensitive probe for the diagnostics of magnetic structures are not clear till now.…”
Section: Introductionmentioning
confidence: 97%
“…Meanwhile, this high surface sensitivity of MSHG is extruded in shadow third-order nonlinear magneto-optical effects because of their bulk localization as well as their small expected value. This is why the observation of magnetization-induced third-harmonic generation (MTHG) is discussed just recently in garnet films [8,9] and magnetic alloys [10]. On the other hand, both the surface MSHG and bulk MTHG are expected to supplement each other as magneto-optical probes and provide complementary information about the magnetic properties of nanostructures.…”
mentioning
confidence: 99%
“…where I 3ω (M ↑↓) are the THG intensities for the opposite directions of the magnetization, χ [8,9] shows that magnetizationinduced variations of the THG intensity result from the internal homodyne effect in the geometry of the transversal Kerr effect (see the left-hand inset in Figure 1, a). To extract the ratio of magnetic and crystallographic components of χ…”
mentioning
confidence: 99%
“…10 In that study, garnet films revealed a rotation of about 4 • and neither the spectral characteristics nor the microscopic origin of the effect were investigated, so that the general aspects of the nature and potential of the TFR remained unclear.…”
Section: B Nonlinear Magneto-optical Rotationmentioning
confidence: 99%