2024
DOI: 10.1021/acs.jpclett.4c02679
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Extracting the Heterogeneous 3D Structure of Molecular Films Using Higher Dimensional SFG Microscopy

Alexander P. Fellows,
Ben John,
Martin Wolf
et al.

Abstract: Ultrathin molecular films are widespread in both natural and industrial settings, where details of the molecular structure such as density, outof-plane tilt angles, and in-plane directionality determine their physicochemical properties. Many of these films possess important molecular-to-macroscopic heterogeneity in these structural parameters, which have traditionally been difficult to characterize. Here, we show how extending sum-frequency generation (SFG) microscopy measurements to higher dimensionality by a… Show more

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