Filling the gaps on the relation between electronic conductivity and catalysis of electrocatalysts for water splitting using computational modelling

Lakhanlal, Lakhanlal; Toroker, Maytal Caspary

doi:10.1016/j.coelec.2023.101342

Current Opinion in Electrochemistry

2023

DOI: 10.1016/j.coelec.2023.101342

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Filling the gaps on the relation between electronic conductivity and catalysis of electrocatalysts for water splitting using computational modelling

Lakhanlal Lakhanlal

Maytal Caspary Toroker

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Cited by 2 publications

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Self‐Supported Earth‐Abundant Carbon‐Based Substrates in Electrocatalysis Landscape: Unleashing the Potentials Toward Paving the Way for Water Splitting and Alcohol Oxidation

Yap,

Loh,

et al. 2023

Advanced Energy Materials

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In the vast realm of scientific inquiry, the pursuit of hydrogen fuel production through electrochemical water splitting offers a promising gateway to green energy generation, alleviating the challenges posed by resource scarcity. However, conventional water splitting encounters hurdles like low efficiency and the sluggish oxygen evolution reaction (OER), which prompt searchers to seek for alternative oxidation process. Significant strides are made in conventional electrocatalytic research employing polymeric binders, resulting in commendable catalytic activity and minimal electron migration resistance. Yet, a pivotal breakthrough in this rapidly evolving field lies in the innovative conception of carbon‐based self‐supported electrocatalysts, heralding a promising trajectory ahead. This review delves into the essential electro‐activity parameters to establish the property‐activity nexus, emphasizing the benefits of self‐supported carbon‐based electrodes. Noteworthy advancements are demonstrated in electrochemical hydrogen evolution reaction (HER), OER, overall water splitting (OWS), and bifunctional HER and alcohol oxidation reaction (AOR), driven by a diverse range of self‐supported electrocatalysts. These include structure‐dependent materials such as metal oxides, hydroxides/oxyhydroxides, phosphides, sulfides, selenides, nitrides, and carbides, each meticulously tailored with nuanced modifications that shape their distinctive attributes. This field also acknowledges its challenges and opportunities, providing guidance for potential research directions and inspiring interdisciplinary collaboration among scientists.

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Self‐Supported Earth‐Abundant Carbon‐Based Substrates in Electrocatalysis Landscape: Unleashing the Potentials Toward Paving the Way for Water Splitting and Alcohol Oxidation

Yap,

Loh,

et al. 2023

Advanced Energy Materials

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Migration-mitigated crossover of organic redox anions across a proton-exchange membrane

Ding,

Vagin,

Jafari

et al. 2024

Sustainable Energy Fuels

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Filling the gaps on the relation between electronic conductivity and catalysis of electrocatalysts for water splitting using computational modelling

Cited by 2 publications

References 76 publications

Self‐Supported Earth‐Abundant Carbon‐Based Substrates in Electrocatalysis Landscape: Unleashing the Potentials Toward Paving the Way for Water Splitting and Alcohol Oxidation

Self‐Supported Earth‐Abundant Carbon‐Based Substrates in Electrocatalysis Landscape: Unleashing the Potentials Toward Paving the Way for Water Splitting and Alcohol Oxidation

Migration-mitigated crossover of organic redox anions across a proton-exchange membrane

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