“…Extensively large amount of work has been done on dye molecule [5][6][7], semiconductor TiO 2 electrodes [8][9][10], counter electrodes [11] and electrolytes [12,13] to improve the DSSCs efficiency and stability. The design of organic dyes (i.e., geometric structures, molecular orbital energy, absorption profiles, and aggregation states of the dye) [14,15], reduction of the rate of charge recombination and the lack of electron donating moiety in the oxidized organic dye have also been proposed to have a great influence on output of DSSCs [16,17]. Thus, there is an intense need to design the molecular structure of organic dye or dye solvents to prevent dye aggregation (Figures 1 and 2).…”