Sodium-aluminium silicates of a high degree of dispersion were obtained. Studies on the surface modi cation of sodium-aluminium silicates using silane coupling agents are described. The best modi ers, which induced a change of the silicate surface from a hydrophilic to a hydrophobic one, were selected. Physicochemical analyses of the obtained silicates were performed. The methods of evaluating the degree of surface modi cation of the silicate are presented. Attempts were made to employ the unmodi ed and modi ed sodium-aluminium silicates as llers in polyurethane elastomers. The introduction of sodium-aluminium silicate into urethane elastomer induced increases in composite parameters such as tensile strength, relative elongation, and hardness. The most pronounced reinforcing effects were observed with urethane elastomers lled with sodium-aluminium silicate modi ed with an aminosilane (A-1120).