Every year the problem of water purification becomes more relevant. This is due to the continuous increase in the level of pollution of natural water sources, an increase in the population, and sharp climatic changes. The growth in demand for affordable and clean water is not always comparable to the supply that exists in the water treatment market. In addition, the amount of water pollution increases with the increase in production capacity, the purification of which cannot be fully handled by conventional processes. However, the application of novel nanomaterials will enhance the characteristics of water treatment processes which are one of the most important technological problems. In this review, we considered the application of carbon nanomaterials in membrane water purification. Carbon nanofibers, carbon nanotubes, graphite, graphene oxide, and activated carbon were analyzed as promising materials for membranes. The problems associated with the application of carbon nanomaterials in membrane processes and ways to solve them were discussed. Their efficiency, properties, and characteristics as a modifier for membranes were analyzed. The potential directions, opportunities and challenges for application of various carbon nanomaterials were suggested.