“…Because external power sources continuously decrease (<3.3 V) and conventional polysilicon floating gate-based flash memory usually adopts 15−25 V for operation, charge trap flash (CTF) memory has drawn intensive attention because of its capability to scale operation voltage. For CTF memory, metal nanocrystals (NCs), such as Au NCs, 1 Ni NCs, 2 W NCs, 3 and TiN NCs, 4 and high-permittivity (high-κ) dielectrics, such as HfO 2 5,6 ZrO 2 , 7,8 ZrON, 9 HfON, 10 HfO 2 /Al 2 O 3 , 11,12 HfO 2 /Si 3 N 4 , 13 and even pure TaN 14 and graphene, 15 have been proposed as the charge-trapping layers. Although these charge-trapping layers realize memory devices with high speed as well as good reliability, the operation voltage is larger than 10 V, and there is still room to reduce the voltage.…”