Herein, we report a general approach to effectively construct C−N or C−C spiroindolines using tetrahydro-βcarbolines as starting materials via a rearrangement coupling reaction. This method is characterized by its operational simplicity and mild conditions. Notably, a wide range of anilines and indoles are suitable for this intermolecular coupling, yielding the corresponding C−N or C−C spiroindolines in good to excellent yields.