2024
DOI: 10.1002/cssc.202401228
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Intrinsically Conductive and Cu‐Functionalized Polymer‐Composite Membranes as Gas Diffusion Electrodes for CO2 Electroreduction

Ignacio Sanjuán,
Vaibhav Kumbhar,
Oleg Prymak
et al.

Abstract: We introduced a new class of gas diffusion electrodes (GDEs) with adjustable pore morphology. We fabricated intrinsically conductive polymer‐composite membranes containing carbon filler, enabling a pore structure variation through film casting cum phase separation protocols. We further selectively functionalized specific pore regions of the membranes with Cu by a NaBH4‐facilitated coating strategy. The as‐obtained GDEs can facilitate the electrochemical CO2 reduction reaction (CO2RR) at Cu active sites that ar… Show more

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