Macrocyclic luminophores under confinement in a polymeric matrix – induction of large-Stokes shift by inter-unit proton transfer

Jurek, Paulina; Rode, Michał F.; Szymański, Marek P.; Banasiewicz, Marzena; Szumna, Agnieszka

doi:10.1039/d3tc01881d

J. Mater. Chem. C

2023

DOI: 10.1039/d3tc01881d

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Macrocyclic luminophores under confinement in a polymeric matrix – induction of large-Stokes shift by inter-unit proton transfer

Paulina Jurek¹,

Michał F. Rode²,

Marek P. Szymański³

et al.

Abstract: We demonstrate that semirigid macrocyclic compounds, tetra(naphthimidazole)resorcin[4]arenes, consisting of four naphthimidazole-resorcinol units, exhibit large bathochromic shifts of emission upon embedding in the polymeric matrix. The mechanism of generation of the...

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2024

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Cited by 2 publications

(1 citation statement)

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“…Compounds 4 , 5 , 7 , and 8 were synthesized previously for a different purpose. 19 The synthesis of 6 and 9 is reported in the ESI †…”

mentioning

confidence: 99%

Remote control of anion binding by CH-based receptors

Jurek,

Szymański,

Szumna

2024

Chem. Commun.

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“…Compounds 4 , 5 , 7 , and 8 were synthesized previously for a different purpose. 19 The synthesis of 6 and 9 is reported in the ESI †…”

mentioning

confidence: 99%

Remote control of anion binding by CH-based receptors

Jurek,

Szymański,

Szumna

2024

Chem. Commun.

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Shining Lights on Limits: Optimizing Luminescent Solar Concentrators for Solar Windows

de Bruin,

van Sark

2024

Advanced Photonics Research

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The luminescent solar concentrator (LSC) can function as an electricity‐generating window whose performance is hindered by an inherent trade‐off between power conversion efficiency and visible light transmission. To optimize this trade‐off, a numerical algorithm is used to find the power conversion efficiency of 92 luminophores, ensuring an average visible transmission >55% and a color rendering index >70. Furthermore, double‐ and triple‐stacked LSC configurations and single LSCs with two‐ or three‐embedded luminophores are optimized. All tested LSC configurations are found to be limited to a power conversion efficiency of around 1% for window‐appropriate transparencies.

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Macrocyclic luminophores under confinement in a polymeric matrix – induction of large-Stokes shift by inter-unit proton transfer

Abstract: We demonstrate that semirigid macrocyclic compounds, tetra(naphthimidazole)resorcin[4]arenes, consisting of four naphthimidazole-resorcinol units, exhibit large bathochromic shifts of emission upon embedding in the polymeric matrix. The mechanism of generation of the...

Cited by 2 publications

References 53 publications

Remote control of anion binding by CH-based receptors

Remote control of anion binding by CH-based receptors

Shining Lights on Limits: Optimizing Luminescent Solar Concentrators for Solar Windows

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