The phase and structural states of nanocrystalline Fe-based films alloyed with Zr and N, which were prepared by reactive magnetron sputtering under different conditions, magnetic-structure parameters of the films and their static and high-frequency magnetic properties have been studied. The interrelation of static magnetic properties and magnetic-structure parameters with the value of real effective magnetic permeability μ’ and frequency range, for which the value is unchanged, has been studied.