2022
DOI: 10.21203/rs.3.rs-1254013/v1
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Manipulation of Rotational States With Varying Pulse Parameter: Achieving High Molecular Alignment and Orientation for CH3F

Abstract: Increasing interest in the fields of high-harmonics generation, laser-induced chemical reactions, and molecular imaging of gaseous targets demands high molecular alignment and orientation (AnO). In this work, we examine the critical role of different pulse parameters on the field-free AnO dynamics of the CH3F molecule, and identify experimentally feasible optical and THz range laser parameters that ensure maximal AnO for such molecules. Herein, apart from rotational temperature, we investigate effects of varyi… Show more

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