Mechanoredox Enabled the Difunctionalization of Unactivated Alkenes via Distal Functional Group Migration

Niu, Sheng-Li; Yuan, Wen; Gong, Xue; Bao, Bo; Wu, Zhi-Wen; Xu, Bo; Zeng, Rong; Yang, Qing-Wu; Ouyang, Qin

doi:10.1021/acssuschemeng.3c06118

ACS Sustainable Chem. Eng.

2023

DOI: 10.1021/acssuschemeng.3c06118

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Mechanoredox Enabled the Difunctionalization of Unactivated Alkenes via Distal Functional Group Migration

Sheng-Li Niu,

Wen Yuan,

Xue Gong

et al.

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2024

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Cited by 4 publications

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Organic Reactions Enabled by Mechanical Force‐Induced Single Electron Transfer

Liu,

He,

Liu

et al. 2024

Chemistry A European J

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Mechanochemical reactions, achieved through milling, grinding, or other mechanical actions, have emerged as a solvent‐free alternative to traditional solution‐based chemistry. Mechanochemistry not only provides the opportunity to eliminate bulk solvent use, reducing waste generation, but also unveils a new reaction strategy which enables the realization of reactions previously inaccessible in solution. While the majority of organic reactions facilitated by mechanical force traditionally follow two‐electron transfer pathways similar to their solution‐based counterparts, the field of mechanochemically induced single‐electron transfer (SET) reactions has witnessed rapid development. This review outlines examples of mechanochemical reactions facilitated by the SET process, focusing on the reagents that initiate SET, thereby positioning mechanochemistry as a burgeoning field within the realm of single‐electron chemistry.

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Organic Reactions Enabled by Mechanical Force‐Induced Single Electron Transfer

Liu,

He,

Liu

et al. 2024

Chemistry A European J

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Mechanochemical Radical Transformations in Organic Synthesis

Sheikhaleslami,

Sperry

2024

Chemistry A European J

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Mechanochemical aerobic oxidative Heck coupling by polymer-assisted grinding: cyclodextrin additive facilitating regioselectivity control

Xiang,

Shou,

et al. 2024

Green Chem.

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Mechanoredox Enabled the Difunctionalization of Unactivated Alkenes via Distal Functional Group Migration

Cited by 4 publications

References 44 publications

Organic Reactions Enabled by Mechanical Force‐Induced Single Electron Transfer

Organic Reactions Enabled by Mechanical Force‐Induced Single Electron Transfer

Mechanochemical Radical Transformations in Organic Synthesis

Mechanochemical aerobic oxidative Heck coupling by polymer-assisted grinding: cyclodextrin additive facilitating regioselectivity control

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