2024
DOI: 10.1002/adfm.202410421
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Metastable Liquid–Liquid Phase Separation and Aging Lead to Strong Processing Path Dependence in Mini‐Spidroin Solutions

Dmitrii Fedorov,
Fred‐Eric Sammalisto,
Adam L. Harmat
et al.

Abstract: Recombinant silk proteins provide a route toward sustainable and biocompatible materials. For making such materials, the assembly process from dilute protein into a functional material is central. The assembly mechanism in engineered materials is by necessity different from the natural ones—this poses challenges but also opens opportunities for scaling up and for developing novel properties. The phase behavior of a mini‐spidroin, NT‐2Rep‐CT is studied, which is a widely studied variant of recombinant silk. NT‐… Show more

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