Human-induced climate change has resulted in long-term drying trends across southern Australia, particularly during the cool season, with the most pronounced impacts observed in the southwest since the 1970s. Although these trends have been linked to changes in large-scale atmospheric circulation features, the limited number of daily weather datasets that extend into the pre-industrial period have so far prevented an assessment of the long-term context of synoptic-level changes associated with global warming. To address this need, we present the development of the longest sub-daily atmospheric pressure, temperature and rainfall records for Australia beginning in 1830. We first consolidate a range of historical observations from the two southern Australian cities of Perth and Adelaide. After assessing the quality and homogeneity of these records, we verify their ability to capture the weather and climate features produced by the Southern Hemisphere’s key climate modes of variability. Our analysis shows the historical observations are sensitive to the influence of large-scale dynamical drivers of Australian climate, as well as the relationship between southwestern and southeastern Australia. Finally, we demonstrate the ability of the dataset to resolve daily weather extremes by examining three severe storms that occurred in the nineteenth century associated with westerly storm tracks that influence southern Australia. The historical dataset introduced here provides a foundation for investigating pre-industrial weather and climate variability in southern Australia, extending the potential for attribution studies of anthropogenically-influenced weather and climate extremes.