“…Among these are the nucleation of mesospheric ice particles (e.g., Rapp and Thomas, 2006), the mesospheric metal chemistry , the D-region charge balance (e.g., Rapp and Lübken, 2001), the heterogeneous formation of water vapour in the mesosphere (Summers et al, 2001), and even the nucleation of polar stratospheric cloud particles which play a major role in the formation of the ozone hole (e.g., Voigt et al, 2005). While some progress regarding the experimental investigation of these atmospheric trace species has been made over the past years with sounding rockets (e.g., Schulte and Arnold, 1992;Gelinas et al, 1998;Horányi et al, 2000;Rapp et al, 2005;Lynch et al, 2005;Barjatya and Swenson, 2006;Amyx et al, 2008;Strelnikova et al, 2009;Rapp et al, 2010), incoherent scatter radars Strelnikova et al, 2007;Fentzke et al, 2009), satellites (Hervig et al, 2009(Hervig et al, , 2012, and laboratory studies (Saunders and Plane, 2006), much of our knowledge about these particles still relies on model results (e.g., Hunten et al, 1980;Gabrielli et al, 2004;Megner et al, 2006Megner et al, , 2008Bardeen et al, 2008).…”