2024
DOI: 10.1021/acscentsci.4c01507
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Multimaterial Thermoset Synthesis: Switching Polymerization Mechanism with Light Dosage

Yuting Ma,
Reagan J. Dreiling,
Elizabeth A. Recker
et al.

Abstract: The synthesis of polymeric thermoset materials with spatially controlled physical properties using readily available resins is a grand challenge. To address this challenge, we developed a photoinitiated polymerization method that enables the spatial switching of radical and cationic polymerizations by controlling the dosage of monochromatic light. This method, which we call Switching Polymerizations by Light Titration (SPLiT), leverages the use of substoichiometric amounts of a photobuffer in combination with … Show more

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