MXene-Based Single-Atom Catalysts for Electrochemical Reduction of CO<sub>2</sub> to Hydrocarbon Fuels

Athawale, A.; Abraham, B. Moses; Jyothirmai, M. V.; Singh, Jayant K.

doi:10.1021/acs.jpcc.3c04732

J. Phys. Chem. C

2023

DOI: 10.1021/acs.jpcc.3c04732

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MXene-Based Single-Atom Catalysts for Electrochemical Reduction of CO₂ to Hydrocarbon Fuels

A. Athawale,

B. Moses Abraham,

M. V. Jyothirmai

et al.

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Cited by 7 publications

References 69 publications

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Emerging Photoreforming Process to Hydrogen Production: A Future Energy

Shelake,

Sutar,

Abraham

et al. 2024

Adv Funct Materials

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In the quest of renewable energy technologies, solar photoreforming emerges as one of the affordable yet challenging process for converting biomass into hydrogen, hydrocarbon fuels, and chemicals. This review highlights the state‐of‐the‐art photoreforming, elucidating its underlying mechanisms for the conversion of dissipated polymers into H2 and valuable chemicals. Biomass feedstocks such as carbohydrates, agricultural residues, glycopolymers, food wastes, and waste plastics are evaluated based on their chemical composition, energy content, and sustainability aspects, exploring the selection of appropriate bio‐renewable resources, considering their abundance, availability, and potential for hydrogen production. The impact of diverse process parameters on photoreforming efficiency is explored, encompassing factors like reaction temperature, pH, catalyst loading, reactor design, solvent effect, and light intensity across various sacrificial substrates. The discussion also considers their correlation with hydrogen production rate, selectivity, and energy efficiency. This review buckles on the design and synthesis of functional photocatalysts for biomass‐derived feedstock, highlighting their photocatalytic (PC) properties in biomass reforming processes and related feedstock into valuable chemicals and biofuel. The review also delves into potential pathways for future advancements including artificial intelligence (AI) and machine learning (ML), alongside addressing the challenges and insightful perspectives within this evolving field of future green energy.

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Emerging Photoreforming Process to Hydrogen Production: A Future Energy

Shelake,

Sutar,

Abraham

et al. 2024

Adv Funct Materials

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Recent Advances in Single‐Atom Catalyst for Solar Energy Conversion: A Comprehensive Review and Future Outlook

Mehmood,

Sk,

Abraham

et al. 2024

Adv Funct Materials

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Single‐atom catalysts (SACs) are becoming increasingly recognized as highly promising catalytic materials, distinguished by their exceptional atomic efficiency, superior selectivity, and elevated activity levels. This review offers a detailed and comprehensive overview of the recent advancements in SACs, focusing on synthesis strategies, photocatalytic energy conversion applications, and advanced characterization techniques. Various synthetic approaches for fabricating atomically dispersed catalysts are elaborated concisely, emphasizing the importance of achieving precise atomic regulation on compatible supports to ensure strong metal–support interactions. Furthermore, the advanced characterization techniques by analytical tools are illustrated for a deep exploration of catalytic activity and mechanistic insights into uniformly dispersed SACs. Specifically, different kinds of support materials such as metal–organic frameworks (MOFs), their subset zeolitic imidazolate frameworks, and graphitic carbon nitride (g‐C3N4) with diverse coordination and electronic environments are examined. Further, advances in computational techniques and machine learning are transforming SACs development by improving predictive accuracy and reducing trial‐and‐error methods, thereby accelerating the discovery of stable and active catalysts. Finally, current challenges and prospects of SACs based on MOFs, and g‐C3N4 are addressed, providing valuable insights for the continued development and application of these catalysts in various industrial processes and environmental remediation efforts.

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Two-dimensional electrode material for (photo)electrochemical reduction of CO2: An overview

Raja,

Chen,

Chen

et al. 2025

International Journal of Electrochemical Science

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MXene-Based Single-Atom Catalysts for Electrochemical Reduction of CO₂ to Hydrocarbon Fuels

Cited by 7 publications

References 69 publications

Emerging Photoreforming Process to Hydrogen Production: A Future Energy

Emerging Photoreforming Process to Hydrogen Production: A Future Energy

Recent Advances in Single‐Atom Catalyst for Solar Energy Conversion: A Comprehensive Review and Future Outlook

Two-dimensional electrode material for (photo)electrochemical reduction of CO2: An overview

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About

MXene-Based Single-Atom Catalysts for Electrochemical Reduction of CO2 to Hydrocarbon Fuels

Cited by 7 publications

References 69 publications

Emerging Photoreforming Process to Hydrogen Production: A Future Energy

Emerging Photoreforming Process to Hydrogen Production: A Future Energy

Recent Advances in Single‐Atom Catalyst for Solar Energy Conversion: A Comprehensive Review and Future Outlook

Two-dimensional electrode material for (photo)electrochemical reduction of CO2: An overview

Contact Info

Product

Resources

About

MXene-Based Single-Atom Catalysts for Electrochemical Reduction of CO₂ to Hydrocarbon Fuels