Natural high-entropy interfaces with kinetics-boosted and water-desolventized effects for high-performance aqueous zinc ion batteries

Li, Yanxin; Jia, Hongfeng; Ali, Usman; Liu, Bingqiu; Li, Lu; Zhang, Lingyu; Wang, Tingting; Wang, Chungang

doi:10.1039/d3gc04298g

Green Chem.

2024

DOI: 10.1039/d3gc04298g

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Natural high-entropy interfaces with kinetics-boosted and water-desolventized effects for high-performance aqueous zinc ion batteries

Yanxin Li,

Hongfeng Jia,

Usman Ali

et al.

Abstract: The degraded performance due to uncontrolled dendrite growth and unfavorable side reactions of the zinc metal anode seriously affects the further application of aqueous zinc ion batteries (ZIBs). In this...

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Design Concepts of High‐Entropy Materials for Zinc Ion Batteries

Sun,

Li,

et al. 2024

Chemistry A European J

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Zinc‐ion batteries have emerged as strong candidates for replacing Li/Na‐ion batteries owing to their high safety and environmental friendliness. However, the large electrostatic repulsion between the cathode and Zn2+, the irreversible growth of zinc dendrites at the anode, and the hydrogen precipitation side reaction in the aqueous electrolyte have hindered the practical application of zinc ion batteries. Fortunately, the emergence of the revolutionary concept of high entropy has provided new opportunities for the development of battery materials. High‐entropy materials, with their unique atomic structures and uniform distribution of multiple elements, offer flexible options for material compositions and electronic structures, thus attracting significant attention in battery systems. In this concept article, we summarize the definitions and intrinsic structural characteristics of high‐entropy materials and provide a detailed overview of the latest design concepts from the perspectives of cathodes, anodes, and electrolytes. Finally, we outline the challenges faced by high‐entropy materials and potential solutions to guide researchers in developing efficient and stable zinc‐ion batteries.

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Design Concepts of High‐Entropy Materials for Zinc Ion Batteries

Sun,

Li,

et al. 2024

Chemistry A European J

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Advanced high-entropy materials for high-quality energy storage and conversion

Fan,

Wang,

et al. 2025

Energy Storage Materials

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Natural high-entropy interfaces with kinetics-boosted and water-desolventized effects for high-performance aqueous zinc ion batteries

Abstract: The degraded performance due to uncontrolled dendrite growth and unfavorable side reactions of the zinc metal anode seriously affects the further application of aqueous zinc ion batteries (ZIBs). In this...

Cited by 2 publications

References 45 publications

Design Concepts of High‐Entropy Materials for Zinc Ion Batteries

Design Concepts of High‐Entropy Materials for Zinc Ion Batteries

Advanced high-entropy materials for high-quality energy storage and conversion

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