“…Deviations between experiment and the calculation based on the simplified model become large at longer wavelengths for which the calculated SHG propagation direction approaches that of the pump. Such deviations are attributed to the influence from the intense pump, the potential mechanism includes the cross-phase-modulation due to pump and SHG coupling [39], parametric scattering [40,41], etc., which were not considered in our calculations. At the incident angle θ = 13 • , the calculated SHG propagation direction is far from that of the pump and the generated SHG intensity is much weaker than other incident angles [ Fig.…”