2024
DOI: 10.1002/ange.202404109
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Non‐Fluorinated Ethers to Mitigate Electrode Surface Reactivity in High‐Voltage NCM811‐Li Batteries

Zhijie Wang,
Xiangli Che,
Danni Wang
et al.

Abstract: Lithium (Li) metal batteries (LMBs) with nickel (Ni)‐rich layered oxide cathodes exhibit twice the energy density of conventional Li‐ion batteries. However, their lifespan is limited by severe side reactions caused by high electrode reactivity. Fluorinated solvent‐based electrolytes can address this challenge, but they pose environmental and biological hazards. This work reports on the molecular engineering of fluorine (F)‐free ethers to mitigate electrode surface reactivity in high‐voltage Ni‐rich LMBs. By me… Show more

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