Optically enhanced coherent transport in YBa2Cu3O6.5 by ultrafast redistribution of interlayer coupling

Hu, W. Z.; Kaiser, Stefan; Nicoletti, D.; Hunt, Cassandra R.; Gierz, Isabella; Hoffmann, Matthias C.; Tacon, M. Le; Loew, T.; Keimer, B.; Cavalleri, Andrea

doi:10.1038/nmat3963

Cited by 401 publications

(479 citation statements)

References 52 publications

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“…An ultrafast (typically femtosecond to picosecond) excitation with a laser pulse or electron beam may cause a transient phase conversion/promotion through electron-electron and/or electron-lattice interactions at the excited state, providing ultrafast control of the electronic state 25 . One of the most amazing phenomena reported recently is the transient photo-creation of possible room-temperature superconductivity in cuprate and C 60 -based superconductors 26,27 .…”

Section: Mottronicsmentioning

confidence: 99%

Emergent functions of quantum materials

2017

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Materials can harbour quantum many-body systems, most typically in the form of strongly correlated electrons in solids, that lead to novel and remarkable functions thanks to emergence-collective behaviours that arise from strong interactions among the elements. These include the Mott transition, high-temperature superconductivity, topological superconductivity, colossal magnetoresistance, giant magnetoelectric e ect, and topological insulators. These phenomena will probably be crucial for developing the next-generation quantum technologies that will meet the urgent technological demands for achieving a sustainable and safe society. Dissipationless electronics using topological currents and quantum spins, energy harvesting such as photovoltaics and thermoelectrics, and secure quantum computing and communication are the three major fields of applications working towards this goal. Here, we review the basic principles and the current status of the emergent phenomena and functions in materials from the viewpoint of strong correlation and topology.E mergence is a concept developed for many-body systems, indicating the properties, phenomena, and functions that never appear in the individual elements but are realized only when a huge number of elements get together 1 . Inside materials, emergent phenomena are often seen due to the interaction of electronic states; with recent developments on electronic states in solids schematically summarized in Fig. 1a. Electrons in solids have several degrees of freedom: charge, spin and orbital, and are characterized by the topological nature determined by the atomic potential on the crystal lattice structure, as schematically shown in Fig. 1b. These five attributes are coupled together and determine the overall responses to stimuli, which appear as materials' electrical, magnetic, optical, thermal, and mechanical properties.These collective electrons demonstrate various macroscopic quantum phenomena, the representative example of which is superconductivity. One of the big challenges in condensed matter physics is to increase the temperature (T c ) at which superconductivity can be observed to above room temperature. However, there are many other macroscopic quantum phenomena that are already observable above room temperature. One is magnetism (by the Bohr-van Leeuwen theorem), and the other is ferroelectricity 2,3 . Remarkably, there are common features of these three macroscopic quantum phenomena: the order parameter, which is of quantum origin, behaves as a classical quantity, and the quantum topology plays a crucial role.The topological nature of the electronic states is the key concept in the most recent developments in understanding quantum materials. The quantum Hall effect, topological insulators, and topological superconductors are all characterized by nontrivial topologies in Hilbert space. The Berry phase, which describes the connection and curvature of the subspace of Hilbert space, plays the central role in the unified principle to describe this topological nature 4 . ...

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Section: Mottronicsmentioning

confidence: 99%

Emergent functions of quantum materials

2017

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“…Moreover, by controlling the light polarization we can negate Volkov states to generate pure Floquet-Bloch states. This work establishes a systematic path for the coherent manipulation of solids via light-matter interaction.The manipulation of solids using ultrafast optical pulses has opened up a new paradigm in condensed matter physics by allowing the study of emergent physical properties that are otherwise inaccessible in equilibrium 1,2,10 . An important example is provided by the Floquet-Bloch states 11 , which emerge in solids owing to a coherent interaction between Bloch states inside the solid and a periodic driving potential.…”

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confidence: 99%

“…The coherent optical manipulation of solids is emerging as a promising way to engineer novel quantum states of matter [1][2][3][4][5] . The strong time-periodic potential of intense laser light can be used to generate hybrid photon-electron states.…”

mentioning

confidence: 99%

“…The manipulation of solids using ultrafast optical pulses has opened up a new paradigm in condensed matter physics by allowing the study of emergent physical properties that are otherwise inaccessible in equilibrium 1,2,10 . An important example is provided by the Floquet-Bloch states 11 , which emerge in solids owing to a coherent interaction between Bloch states inside the solid and a periodic driving potential.…”

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confidence: 99%

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Selective scattering between Floquet–Bloch and Volkov states in a topological insulator

Mahmood¹,

Chan²,

Alpichshev³

et al. 2016

Nature Phys

339

273

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The coherent optical manipulation of solids is emerging as a promising way to engineer novel quantum states of matter 1-5 . The strong time-periodic potential of intense laser light can be used to generate hybrid photon-electron states. Interaction of light with Bloch states leads to Floquet-Bloch states, which are essential in realizing new photo-induced quantum phases [6][7][8] . Similarly, dressing of free-electron states near the surface of a solid generates Volkov states, which are used to study nonlinear optics in atoms and semiconductors 9 . The interaction of these two dynamic states with each other remains an open experimental problem. Here we use time-and angle-resolved photoemission spectroscopy (Tr-ARPES) to selectively study the transition between these two states on the surface of the topological insulator Bi 2 Se 3 . We find that the coupling between the two strongly depends on the electron momentum, providing a route to enhance or inhibit it. Moreover, by controlling the light polarization we can negate Volkov states to generate pure Floquet-Bloch states. This work establishes a systematic path for the coherent manipulation of solids via light-matter interaction.The manipulation of solids using ultrafast optical pulses has opened up a new paradigm in condensed matter physics by allowing the study of emergent physical properties that are otherwise inaccessible in equilibrium 1,2,10 . An important example is provided by the Floquet-Bloch states 11 , which emerge in solids owing to a coherent interaction between Bloch states inside the solid and a periodic driving potential. This is a consequence of the Floquet theorem 12 , which states that a Hamiltonian periodic in time with period T has eigenstates that are evenly spaced by the drive energy (2π/T ). Floquet-Bloch states have generated a lot of interest recently both for realizing exotic states of matter such as a Floquet Chern insulator 7 , as well as understanding non-equilibrium periodic thermodynamics 13,14 . Experimental observation of these states requires the measurement of the transient electronic band structure of a crystal as it is perturbed by light. As has recently been demonstrated 15 in the topological insulator Bi 2 Se 3 , time-and angleresolved photoemission spectroscopy (Tr-ARPES) is a key tool that can achieve this. Characteristic signatures of Floquet-Bloch states in the Tr-ARPES spectra include replicas of the original band structure that are separated by the driving photon energy 15 .In addition to Floquet-Bloch states, light can also generate other coherent phenomena in solids [16][17][18] . In particular, it can dress freeelectron states near the surface of a solid (Fig. 1a), as the surface can provide the momentum conservation necessary for a photon to interact with a free electron. This dressing was first observed in time-resolved photoemission experiments 17 and has subsequently been referred to as laser-assisted photoemission (LAPE). LAPE is typically understood [19][20][21] by invoking the Volkov solution, which is an e...

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“…Different tools have been developed for different experimental systems. Important examples are various cold-atom setups [1][2][3][4][5][6] , ultra-fast pump-probe spectroscopy of quantum materials [7][8][9][10] , and heavy-ion collisions that explore the dynamics of the quark-gluon plasma 11 . These experiments clearly reveal that observations far away from equilibrium can yield new insights.…”

Section: Introductionmentioning

confidence: 99%

Universal postquench coarsening and aging at a quantum critical point

2015

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The non-equilibrium dynamics of a system that is located in the vicinity of a quantum critical point is affected by the critical slowing down of order-parameter correlations with the potential for novel out-of-equilibrium universality. After a quantum quench, i.e. a sudden change of a parameter in the Hamiltonian such a system is expected to almost instantly fall out of equilibrium and undergo aging dynamics, i.e. dynamics that depends on the time passed since the quench. Investigating the quantum dynamics of a N -component ϕ 4 -model coupled to an external bath, we determine this universal aging and demonstrate that the system undergoes a coarsening, governed by a critical exponent that is unrelated to the equilibrium exponents of the system. We analyze this behavior in the large-N limit, which is complementary to our earlier renormalization group analysis, allowing in particular the direct investigation of the order-parameter dynamics in the symmetry broken phase and at the upper critical dimension. By connecting the long time limit of fluctuations and response, we introduce a distribution function that shows that the system remains non-thermal and exhibits quantum coherence even on long timescales.

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Optically enhanced coherent transport in YBa2Cu3O6.5 by ultrafast redistribution of interlayer coupling

Cited by 401 publications

References 52 publications

Emergent functions of quantum materials

Emergent functions of quantum materials

Selective scattering between Floquet–Bloch and Volkov states in a topological insulator

Universal postquench coarsening and aging at a quantum critical point

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