2024
DOI: 10.1002/adfm.202413134
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Oxophilic Low‐Coordination Gd‐N3 Single Atom Sites With P‐Enhanced Second Coordination for High‐Performance Al‐Air Batteries

Yan Liu,
Lei Zhang,
Qiaoling Xu
et al.

Abstract: The development of efficient rare earth single‐atom (SA) catalysts for the oxygen reduction reaction (ORR) is essential yet challenging for high‐performance aluminum‐air batteries (AABs). This study introduces a concept‐to‐proof strategy for synthesizing a hollow carbon‐supported gadolinium (Gd) SA catalyst using low‐coordination and second‐coordination sphere engineering. In this design, Gd atoms are coordinated to three nitrogen (N) atoms in N‐doped carbon and surrounded by six phosphorus (P) atoms, forming … Show more

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