2021
DOI: 10.1002/ange.202105343
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Partial Coordination‐Perturbed Bi‐Copper Sites for Selective Electroreduction of CO2 to Hydrocarbons

Abstract: In the electrochemical CO2 reduction reaction (CO2RR), it is challenging to develop a stable, well‐defined catalyst model system that is able to examine the influence of the synergistic effect between adjacent catalytic active sites on the selective generation of C1 or C2 products. We have designed and synthesized a stable crystalline single‐chain catalyst model system for electrochemical CO2RR, which involves four homomorphic one‐dimensional chain‐like compounds (Cu‐PzH, Cu‐PzCl, Cu‐PzBr, and Cu‐PzI). The mai… Show more

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Cited by 5 publications
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