Pd‐Imidate@Sba‐15: A Multifunctional Heterogeneous Catalyst for the Aqueous Room Temperature Hydrogenation of Co2 to Formic Acid
Nuria Martín,
Raúl Porcar,
José L. Serrano
et al.
Abstract:The incorporation of hydrophilic and basic sites from phosphotriazaadamantane and saccharine in a water‐soluble Pd complex and the subsequent confinement into mesoporous silica support increases the activity and stability of the palladium catalytic species for the room‐temperature aqueous hydrogenation of either bicarbonate or CO2 into formic acid. The use of low Pd loadings (<0.1mmolPd·g‐1) of the well‐dispersed complex on SBA‐15 mesoporous silica allows performing the reaction under room temperature, and … Show more
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