2023
DOI: 10.1021/acs.energyfuels.3c03268
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Perylenediimide-Incorporated Covalent Triazine Framework: A Highly Conductive Carbon Support for Copper Single-Atom Catalysts in Electrocatalytic CO2 Conversion

Sebastian Raja,
Gelson T. S. T. da Silva,
Eduardo A. Reis
et al.

Abstract: Here, we show that a perylenediimide-incorporated covalent triazine framework (PDI-CTF) leads to an adequate conductive carbon support for copper single-atom catalysts (Cu-SACs), allowing the selective electroreduction of CO2 to methanol. CTF-Cu-SACs converted CO2 into methanol with a faradaic efficiency of 72.6% at a low overpotential (0.2 V vs RHE). While increasing the overpotential (0.2 to −0.4 V vs RHE), CTF-Cu-SACs promoted syngas (CO and H2) production with faradaic efficiencies of 53.2 and 39.5%, respe… Show more

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