“…Temporally, the concentration levels of TOC and PAHs in wet deposition from the present study were lower than those from previous studies also conducted in Guangzhou, i.e., the level of TOC in 2010 (2.5 mg L À1 ) was lower than those in 2004 (7.1 mg L À1 ) (Xu et al, 2008) and levels of PAHs in 2010 (170 ng L À1 ) were lower than those in 2005 (1910 ng L À1 ). On the other hand, the relative abundance of the low molecular weight (3 þ 4-ring) PAHs, mainly derived from low-efficient combustion of domestic coal and biomass (Liu et al, 2012b), was reduced from 86% in 2005 to 61% in 2010 (Huang et al, 2009 or > 0.5 and in the range of 0.2e0.35 or 0.2e0.5 indicate coal or wood burning and petroleum combustion, respectively (Yunker et al, 1996(Yunker et al, , 2002. In the present study, the mean values of these two indices both decreased from 2005 (0.37 and 0.53) (Huang et al, 2009) to 2010 (0.29 and 0.46), uniformly suggesting similar , and those of straw decreased 69% (68%).…”