“…Since the first invention of M41s series of silica materials [ 1 , 2 ], ordered mesoporous materials possessing large pore volume and high specific surface area as well as tunable mesoporous structures have attracted extensive attention for the development of high-efficiency catalysts using in the conversion of macromolecules [ 3 ], and numerous non-silicon-based ordered mesoporous materials with excellent structural, textural, and surface properties have been successively synthesized [ 4 , 5 , 6 , 7 ]. Compared to ordered mesoporous silica materials, ordered mesoporous alumina materials as catalysts or catalyst supports exhibit much more broad application prospects in various petrochemical processes, including hydrodesulfurization, cracking, and hydrocracking of petroleum feedstocks [ 8 , 9 , 10 , 11 , 12 ], because of the thoughtful combination of both the chemical properties of alumina and ordered mesoporous characteristics.…”