2021
DOI: 10.48550/arxiv.2111.09090
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Purifying single photon emission from giant shell CdSe/CdS quantum dots at room temperature

Abstract: Colloidal quantum dots are robust and flexible single photon emitters for room-temperature applications, but their purity is strongly reduced at high pump powers, due to multiexcitonic emission which cannot be easily filtered due to the photo-luminescence spectral broadening at room temperature. Giant-shell quantum dots feature a large blueshift of the biexciton spectrum due to electron-hole wave function engineering and piezoelectric charge separation, which can be exploited for spectral separation of the sin… Show more

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