“…Here, on the basis of literature precedent, 29,32 we use n m ) 1, while n 1 ) 1 and n 2 ) 1.51 near 800-860 nm, and 1.53 around 400-430 nm. Finally, the nonlinear susceptibility, χ (2) , can be expressed as the linear combination of the molecular nonlinear polarizability, β, by where i, j, and k are laboratory coordinates and l, m, and n are molecular coordinates. ML(θ,φ,ψ) is the molecular-to-laboratory frame (Euler angle) transformation matrix and can be expressed as follows:…”