Regulating Interfacial Hydrogen‐Bonding Networks by Implanting Cu Sites with Perfluorooctane to Accelerate CO2 Electroreduction to Ethanol
Jing Zhou,
Bingling He,
Pu Huang
et al.
Abstract:Efficient CO2 electroreduction (CO2RR) to ethanol holds promise to generate value‐added chemicals and harness renewable energy simultaneously. Yet, it remains an ongoing challenge due to the competition with thermodynamically more preferred ethylene production. Herein, we presented a CO2 reduction predilection switch from ethylene to ethanol (ethanol‐to‐ethylene ratio of ~5.4) by inherently implanting Cu sites with perfluorooctane to create interfacial non‐covalent interactions. The 1.83%F‐Cu2O organic‐inorgan… Show more
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