Abstract:The present investigation observed the effect of current density (CD), operating time (OT), inter electrode distance (IED), electrode area (EA), initial pH and settling time (ST) using Al-Al electrode combination on the removal of color, total suspended solids (TSS), hardness (HR) and alkalinity (ALK) from biologically treated municipal wastewater (BTMW) of Sewage Treatment Plant (STP), Jagjeetpur, Haridwar, India. The maximum removal of color (99.86%), TSS (98.7%), HR (78.9%) and ALK (43.69 %) from BTMW was found with the optimum operating conditions of CD (2.65 A/m 2 ), OT (40 mins.), IED (0.5 cm), EA (160 cm 2 ), initial pH (7.5) and ST (60 min.). However, the maximum removal of ALK was found with the optimum operating conditions of CD (1.68 A/m 2 ), OT (40 mins.), IED (1.0 cm), EA (80 cm 2 ), initial pH (7.5) and ST (90 min.) The electrolytic treatment ( ET) brought down the concentration of HR and ALK to the desirable limit of the BIS standards of drinking water. There was no need of pH adjustment of the BTMW during ET as the optimal removal efficiency was close to the pH of 7.5. Under optimal operating conditions, the operating cost was found to be 1.01 $/m 3 in terms of the electrode consumption (23. ). The study revealed that BTMW can be effectively treated with the Al-Al electrode combination for color, TSS, HR and ALK removal.