Resonance Raman and Optical Dephasing Study of Hitci

Abstract

Line shape analysis based on resonance Raman spectra of HITCI is used to determine the details of the vibrational part of the line broadening function. Forced Light Scattering with 20 fs pulses from a Ti: sapphire laser measured optical dephasing probing with an Ar laser. The observed response is well described by the line broadening function derived from the fluorescence line shape.