“…In that fitting, the polarization relaxation rate of the medium had to be cited from other literature. In this paper, we developed a new method to measure the dynamical parameters independently by using the laser cavity modulation process [2]. The laser dynamics is described by the reduced equations including vibro-rotational levels [3] dI/dt = where I and D are the suitably normalized variables for the laser intensity and the population difference between upper and lower laser levels, respectively, with decay rates 2 K and y II (we use K for the decay rate of the electric field in the laser cavity).…”