2024
DOI: 10.1002/adfm.202419656
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Rigid Additives Enabling Inorganic‐Rich Interphase via Steric Effects and Van der Waals Force for Stable Lithium Metal Batteries

Shuhao Yao,
Chi Guo,
Yuxi Yang
et al.

Abstract: Electrolyte additives (EAs) are cost‐effective for stabilization of lithium metal batteries (LMBs). Nevertheless, most EAs are gradually consumed during the lithium deposition process, rendering them inadequate for long‐term cyclability. Herein, a novel hybrid metal–organic framework (MOF)‐based non‐expendable additive is prepared through polymerization of pentaerythritol tetraacrylate (PETEA) on a zeolitic imidazolate framework (ZIF‐67). Owing to the partial coating by PETEA‐based polymer, the exposed unsatur… Show more

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