“…Therefore, the reported composition and size of droplet residuals are expected to be representative of the entire droplet population, since larger droplets are not necessarily associated with more hygroscopic and/or larger residual particles. 57 Aerosol size distributions (mobility diameter, d m ) in the size range from 10 nm to 0.4 mm were measured using a fast integrated mobility spectrometer (FIMS) 58 and used to quantify total particle number concentrations and concentration of particles in accumulation mode (with diameters >0.1 mm). Cloud condensation nuclei (CCN) measurements were performed using a cloud condensation nuclei counter (CCNC, DMT), 59 operating at two instrument supersaturations: 0.24% and 0.46%.…”