2024
DOI: 10.1002/ange.202414180
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Small‐Molecule Mixed Ionic‐Electronic Conductors for Efficient N‐Type Electrochemical Transistors: Structure‐Function Correlations

Yongjoon Cho,
Lin Gao,
Yao Yao
et al.

Abstract: The fundamental challenge in electron‐transporting organic mixed ionic‐electronic conductors (OMIECs) is simultaneous optimization of electron and ion transport. Beginning from Y6‐type/U‐shaped non‐fullerene solar cell acceptors, we systematically synthesize and characterize molecular structures that address the aforementioned challenge, progressively introducing increasing numbers of oligoethyleneglycol (OEG; g) sidechains from 1g to 3g, affording OMIECs 1gY, 2gY, and 3gY, respectively. The crystal structure … Show more

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