2024
DOI: 10.1002/smll.202401392
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Solvated Electrons Generated on the Surface of Na‐SPHI for Boosting Visible Light Photocatalytic Hydrogen Evolution with Ultra‐High AQE

Yuxuan Li,
Dachuan Ge,
Hui Zhang
et al.

Abstract: Enhancing the utilization of visible‐light‐active semiconductors with an excellent apparent quantum efficiency (AQE) remains a significant and challenging goal in the realm of photocatalytic water splitting. In this study, a fully condensed sulfur‐doped poly(heptazine imide) metalized with Na (Na‐SPHI) is synthesized by an ionothermal method by using eutectic NaCl/LiCl mixture as the ionic solvent. Comprehensive characterizations of the obtained Na‐SPHI reveal several advantageous features, including heightene… Show more

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