2022
DOI: 10.26434/chemrxiv-2022-69z8f
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Straightforward access to multifunctional pi-conjugated P-heterocycles

Abstract: We report the straightforward one-pot synthesis of 5 or 6-membered P-heterocycles featuring internal ylidic bond: P-containing acenaphthylenes and phenanthrenes. The stability of the compounds tolerates post-functionalization through direct arylation to introduce electron-rich/poor substituents and the synthetic strategy is also compatible with the preparation of more elaborated polyaromatic scaffolds such acenes and helicenes. Using a joint experimental and theoretical approach, we show that the molecular eng… Show more

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